No, this construction is impossible because it has nominal syntax (hoc domūs tēctum "the roof of this house""this house roof") like the English gerund, while the Latin gerund has verbal syntax (not *in hōc scrībendō "in this writing") and governs the same case as the verb (not *epistolārum scrībere "to write of letters"-letters"). With verbs that govern the genitive, in whichwhere it expresses the stimulus that evokes some feeling (memory, pity, incrimination), you can say:
- eōs prūdentiae monēmus > tempus perdimus eōs prūdentiae monendō ('to warn them of discretion > we waste time warning them of discretion').
Other than that, suchnominal syntax with a gerund is probably impossible even in Late Latin, where hoc epistolārum scrībere "this writing of letters"letters, this letter-writing" becomes grammatical. That said, due to the suppletive relationship1 between the infinitive and the gerund, it wouldn't surprise me to find a substantive-like prepositional use, eg. *?in epistolārum scrībendō in Late/Medieval Latin.
1: the infinitive serves as the nominative of the gerund.
In the Cicero quote, operae is the partitive genitive that depends on plūs as the object of pōnere: 'to put in more work.'